You need an original ROM file, and this here, according to the article.
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Not sure about Perfect Dark (never played it), but Goldeneye had the control mode where you hold the left and center grips which was quite similar to dual analog. Of course, that was moving with the d-pad instead of moving with an analog stick, so not quite as smooth on the movement front, but it was definitely a step up from the default control scheme while not being quite as unwieldy as using two separate controllers.
Turok had you use the c buttons for movement and the stick to aim. It worked really well, and was functionally dual-analog too.